http://www.braingle.com/
http://www.sharpbrains.com/teasers/brain-games-the-latest/
http://www.scilearn.com/products/brainapps/lunar-tunes/index.php Lunar Tunes is an exercise that will test your auditory and visual-spatial memory.
http://www.scilearn.com/products/brainapps/hoop-nut/index.php Hoop Nut is an exercise that will test your auditory processing speed and ability to focus your attention.
Radica Brain Games
The iBrain book also suggests some low tech ideas like learning how to play chess, taking up the tuba and volunteering at a local hospital. Maybe 2009 is the year to learn a foreign language, as well?